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- W2149079557 abstract "The N-heterocyclic carbene (NHC)-catalyzed generation of chiral α,β-unsaturated acylazoliums from 2-bromoenals followed by their interception with 1,3-dicarbonyl compounds or enamines, the formal [3+3] annulation reaction, is reported. The reaction results in the enantioselective synthesis of synthetically and medicinally important dihydropyranones and dihydropyridinones, and tolerates a wide range of functional groups. It is noteworthy that the reaction takes place under mild reaction conditions utilizing relatively low catalyst loadings. In addition, based on DFT calculations, a mechanistic scenario involving the attack of the nucleophile from below the plane of the α,β-unsaturated acylazoliums, and the mode of enantioinduction is presented." @default.
- W2149079557 created "2016-06-24" @default.
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- W2149079557 date "2013-04-08" @default.
- W2149079557 modified "2023-10-15" @default.
- W2149079557 title "Enantioselective N-Heterocyclic Carbene-Catalyzed Annulations of 2-Bromoenals with 1,3-Dicarbonyl Compounds and Enamines<i>via</i>Chiral α,β-Unsaturated Acylazoliums" @default.
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- W2149079557 doi "https://doi.org/10.1002/adsc.201300219" @default.
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