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- W2149170837 abstract "Abstract As a case study, the energy landscape of the cesium chloride/lithium chloride system was investigated by combining theoretical and experimental methods. Global optimization for many compositions of this quasi‐binary system gave candidates for possible modifications that constitute promising targets for subsequent syntheses based on solid‐state reactions. Owing to the synergetic and complementary nature of the computational and experimental approaches, a substantially better efficiency of exploration was achieved. Several new phases were found in this system, for the compositions CsLiCl 2 and CsLi 2 Cl 3 , and their thermodynamic ranking with respect to the already‐known phases was clarified. In particular, the new CsLiCl 2 modification was shown to be the low‐temperature phase, whilst the already‐known modification for this composition corresponded to a high‐temperature phase. Based on these results, an improved cesium chloride/lithium chloride phase diagram was derived, and this approach points the way to more rational and more efficient solid‐state synthesis." @default.
- W2149170837 created "2016-06-24" @default.
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- W2149170837 date "2012-02-23" @default.
- W2149170837 modified "2023-10-18" @default.
- W2149170837 title "Theoretical and Experimental Exploration of the Energy Landscape of the Quasi-Binary Cesium Chloride/Lithium Chloride System" @default.
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- W2149170837 doi "https://doi.org/10.1002/chem.201103162" @default.
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