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• W2149267075 startingPage "976" @default.
• W2149267075 abstract "The change of sign with composition in aqueous mixtures of associating fluids is analyzed by means of molecular-dynamics simulations. The results obtained are in quantitative agreement with the experimental data in water-ethanol and water-methanol solutions, which exhibit the mentioned change of sign. A subsequent theoretical analysis is addressed to establish a relationship between the dependence of the Soret coefficient with composition with the existence of large inter-species interactions. Although the change of sign of the Soret coefficient with composition is not only due to the so-called chemical contribution analyzed here, we discuss the role that these interactions play in such a change of sign." @default.
• W2149267075 created "2016-06-24" @default.
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• W2149267075 date "2004-09-01" @default.
• W2149267075 modified "2023-10-17" @default.
• W2149267075 title "The role of molecular interactions in the change of sign of the Soret coefficient" @default.
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• W2149267075 doi "https://doi.org/10.1209/epl/i2004-10136-3" @default.
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