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- W2149309416 abstract "Wir beschreiben die Herstellung und das Hydrierungsverhalten eines Einzelatom-Palladiumkatalysators, geschaffen durch die Verankerung von Pd-Atomen in den Mesoporen eines graphitischen Kohlenstoffnitridpolymers. Die Analyse des Materials bestatigt die atomare Dispersion der Palladium-Phase uber die komplette Probe. Gegenuber nanopartikelbasierten Vergleichskatalysatoren zeigte sich die hohe Aktivitat und Selektivitat deutlich bei Anwendung in der kontinuierlichen Drei-Phasen-Hydrierung von Alkinen und Nitroarenen in einem Durchflussreaktor. Dichtefunktionalrechnungen ermoglichten die Erarbeitung fundamentaler Erkenntnisse betreffend Materialstruktur und erlaubten, die hohe katalytische Aktivitat und Selektivitat auf die einfache Wasserstoffaktivierung und Kohlenwasserstoffadsorption auf den atomar verteilten Pd-Strukturen zuruckzufuhren." @default.
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- W2149309416 date "2015-07-31" @default.
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- W2149309416 title "Ein stabiler “Single-site”-Palladiumkatalysator für Hydrierungen" @default.
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- W2149309416 doi "https://doi.org/10.1002/ange.201505073" @default.
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