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• W2149339954 abstract "The decomposition products of the d6-ethane cation following charge-transfer ionization with Ar+, under conditions of varying ionization electron current, have been isolated in solid argon matrices at 18 K and examined using Fourier transform infrared spectroscopy. Gas samples containing 1 : 1600 d6-ethane : Ar were subjected to electron bombardment by using either a high (pin) or a low (plate) ionization density anode configuration with ionization currents between 20 and 150 μA. Under high ionization density conditions, the observed major products were d4-ethene (C2D4) and d2-acetylene (C2D2), with smaller yields of C2D5, C2D3, and C2D. The yield of each dehydrogenation product was enhanced with increased current. Analogous experiments employing the low ionization density plate anode resulted in reduced C2D6 destruction and the formation of only C2D4 and C2D2. The results suggest the onset of dissociative recombination processes under high ion density conditions. In this context, the results can be interpreted as a dissociative recombination of primary ion products, which gives rise to further dehydrogenation, and appearance of additional neutral radical products. Copyright © 2012 John Wiley & Sons, Ltd." @default.
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• W2149339954 date "2012-01-01" @default.
• W2149339954 modified "2023-09-26" @default.
• W2149339954 title "Ethane cation decomposition characterization by EBMI spectroscopy: gas-phase dissociative recombination as a source of secondary products" @default.
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• W2149339954 doi "https://doi.org/10.1002/jms.2030" @default.
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