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- W2149366457 abstract "Two-photon photoacoustic spectra of acetone-h6 and −d6 have been recorded using a pulsed laser in the 3p←n Rydberg transition region (332.2–338.7 nm for two-photon excitation). Comparison of the acetone-h6 and −d6 photoacoustic and two-photon resonance enhanced multiphoton ionization spectra shows an intensity reversal between the (3py←n)1A1 and (3px←n)1A2 transition origins. The dramatic increase in the 1A1 state - and to a lesser extent for the 1B2 state - photoacoustic signals requires efficient radiationless/dissociative channels for these states, not present for 1A2. The intensity effects are interpreted through the 1A1 state having substantial π*←π valence character in contrast to almost pure Rydberg character for the 1A2 state." @default.
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- W2149366457 date "1992-11-01" @default.
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- W2149366457 title "Two-photon photoacoustic spectroscopy of acetone 3p Rydberg states" @default.
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- W2149366457 doi "https://doi.org/10.1016/0009-2614(92)80128-x" @default.
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