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- W2149366997 abstract "Abstract Mn x Zn (1− x ) CO 3 solid-solutions were prepared at 5°C by precipitation from metal-bearing bicarbonate solutions. The solids were identified by X-ray powder diffraction and infrared spectroscopy. Zn 2+ ions substitute extensively for Mn 2+ ions in the crystal lattice of anhydrous rhombohedral carbonates. Throughout the 24 h during which the experiments were conducted, the aqueous solutions remained undersaturated with respect to pure oxides, sulphates, hydroxides and hydroxysulphates. The solutions, however, were supersaturated with Mn x Zn (1− x ) CO 3 of any given composition. Besides the anhydrous rhombohedral carbonates, Zn 4 (OH) 2 (CO 3 ) 3 ·4H 2 O was precipitated from an aqueous solution with initially high Zn 2+ concentration. The negative logarithm of the solubility product of Zn 4 (OH) 2 (CO 3 ) 3 ·4H 2 O was estimated theoretically to be 43.9 (25°C). Remaining saturation with respect to Zn 4 (OH) 2 (CO 3 ) 3 ·4H 2 O was calculated accordingly. The suggestion is made that hydrated zinc hydroxycarbonate is metastable under the experimental conditions used here, but that it should transform into anhydrous carbonates." @default.
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- W2149366997 date "1995-09-01" @default.
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- W2149366997 title "The formation of rhodochrosite–smithsonite (MnCO<sub>3</sub>–ZnCO<sub>3</sub>) solid-solutions at 5°C" @default.
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