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- W2149627690 abstract "We developed the synthesis of a multicomponent molecular machine by employing the inclusion complex of an azobenzene-containing pyridinium salt (G1) with α-cyclodextrin (α-CD) and tetrasulfonated 1,5-dinaphtho-32-crown-8 (DNC) in water. The interconversion of the heterowheel trans-G1⋅DNC⋅α-CD [3]pseudorotaxane into cis-G1⋅DNC [2]pseudorotaxane was modulated by the photoinduced isomerization of the azobenzene moiety accompanied by the release of α-CD from the molecular axle. In control experiments, the azobenzene center of the bis(pyridinium)-modified azobenzene (G2) could not be isomerized in the presence of DNC and α-CD. Only polymeric aggregates were obtained with the G2⋅DNC⋅α-CD system, which indicates that the inclusion complex with α-CD and the electrostatic attraction with DNC are crucial to govern the reversible photoswitchable process. This work may provide a method to induce conformational changes of supramolecular assemblies that have multiple macrocyclic receptors." @default.
- W2149627690 created "2016-06-24" @default.
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- W2149627690 date "2015-01-15" @default.
- W2149627690 modified "2023-09-27" @default.
- W2149627690 title "Light-Controlled [3]Pseudorotaxane Based on Tetrasulfonated 1,5-Dinaphtho-32-Crown-8 and α-Cyclodextrin" @default.
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- W2149627690 doi "https://doi.org/10.1002/ajoc.201402238" @default.
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