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- W2150025229 abstract "Transient resonance coherent Stokes Raman scattering (CSRS) spectra of the photoinduced radical ions of all-trans-1, 8-diphenylocta-1, 3, 5, 7-tetraene (DPO) were observed in polar solvents such as acetonitrile, N, N-dimethylformamide and dimethyl sulphoxide. The identification was based on the long lifetimes and the dependence of their formation on the electron-donating and/or -accepting nature of the solvents. The fluorescence spectra of DPO were also observed in the presence of N, N-dimethylaniline (DMA) and p-dicyanobenzene (DCNB) in p-dioxane and in polar solvents without DCNB and DMA. The absence of an indication of exciplex formation, in contrast to the cases of diphenylbutadiene and diphenylhexatriene, can be related to the extremely low efficiency of the radical ion formation by solvent-assisted photoionization in DPO—DMA and DPO—DCNB in p-dioxane systems. The strong dependence of the CSRS signal of the DPO radical ions on the content of polar solvent in the high-concentration region of the binary solvent systems with p-dioxane suggests a collective behaviour of the polar solvents surrounding an S1 solute for the CT interaction to generate the radical ions. The observed Raman wavenumbers were compared with those of DPO in the S0, S1 and T1 states and qualitative correlation among them is discussed." @default.
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- W2150025229 date "1995-01-01" @default.
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- W2150025229 title "Transient resonance coherent stokes Raman scattering spectra of photoinduced radical ions of diphenyloctatetraene in polar solvents" @default.
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- W2150025229 doi "https://doi.org/10.1002/jrs.1250260114" @default.
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