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- W2150324039 abstract "The Raman spectra of a series of monolayer-protected gold clusters were investigated with special emphasis on the Au–S modes below 400 cm–1. These clusters contain monomeric (SR-Au-SR) and dimeric (SR-Au-SR-Au-SR) gold–thiolate staples in their surface. In particular, the Raman spectra of [Au25(2-PET)18]0/–, Au38(2-PET)24, Au40(2-PET)24, and Au144(2-PET)60 (2-PET = 2-phenylethylthiol) were measured in order to study the influence of the cluster size and therefore the composition with respect to the monomeric and dimeric staples. Additionally, spectra of Au25(2-PET)18–2x(S-/rac-BINAS)x (BINAS = 1,1′-binaphthyl-2,2′-dithiol), Au25(CamS)18 (CamS = 1R,4S-camphorthiol), and AunBINASm were measured to identify the influence of the thiolate ligand on the Au–S vibrations. The vibrational spectrum of Au38(SCH3)24 was calculated which allows the assignment of bands to vibrational modes of the different staple motifs. The spectra are sensitive to the size of the cluster and the nature of the ligand. Au–S–C bending a..." @default.
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- W2150324039 date "2014-04-23" @default.
- W2150324039 modified "2023-09-26" @default.
- W2150324039 title "Structural Information on the Au–S Interface of Thiolate-Protected Gold Clusters: A Raman Spectroscopy Study" @default.
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- W2150324039 doi "https://doi.org/10.1021/jp502453q" @default.
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