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• W2150962776 abstract "Abstract The CH functionalization of methane by means of direct CH borations with BH 3 or MeBH 2 is compared computationally (using the B3LYP/6‐311 ++ G** method) to CH lithiations with LiH or LiMe as well as to other analogue C–metal (Be, Na, Mg, Al) formations. For the borations only, this internal electrophilic substitution at carbon (S E i) relies more on the electrophilicity of boron than on the basicity of the internal base Y, that is, H or Me. Such direct borations of methane are more favored for dehydrogenations than for dehydrocarbonations. Due to decreased electrophilicity, substituents at boron disfavor such borations. Hence, the BH 2 group appears to be most efficient for CH functionalizations by means of direct hydrocarbon borations." @default.
• W2150962776 created "2016-06-24" @default.
• W2150962776 creator A5008760753 @default.
• W2150962776 date "2009-11-18" @default.
• W2150962776 modified "2023-10-18" @default.
• W2150962776 title "CH Functionalizations by Means of Direct Borane–Hydrocarbon Dehydrogenations and Dehydrocarbonations" @default.
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• W2150962776 doi "https://doi.org/10.1002/chem.200901368" @default.
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