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- W2151486750 abstract "Diffusion coefficients (D) of polychlorinated biphenyls (PCBs) and polycyclic aromatic hydrocarbons (PAHs) were determined by film-stacking technique in low-density polyethylene (LDPE) and two types of polydimethylsiloxane (PDMS) (also known as silicone rubber, SR) with the trade names AlteSil™ and Silastic®. The estimated values of D for PCBs and PAHs over a wide range of hydrophobicity were 2–2.5 orders of magnitude lower in LDPE than in SR polymers. Log D (m2 s−1) of PCBs ranged from −10.1 to −10.9 for SRs and from −12.4 to −13.7 for LDPE. For PAHs these ranges were −9.8 to −11.4 for SRs and −11.9 to −13.7 for LDPE. Compared with the D values calculated in water, D were 1–2 and 3–4 orders of magnitude lower in SR and LDPE, respectively. For PAH molecules, D was lower than for PCBs with a similar molecular weight, probably because of their more rigid structure. The range of log D for PCBs in SR was only 0.5 log units (factor of 3.2) versus 1.2 log units (factor of 16) in LDPE. Although compound classes showed different relations, a linear relation of D with total surface area was the most universal. This relation may be used for prediction of D values in SR and LDPE polymers for other organic compounds. © 2010 Wiley Periodicals, Inc. J Appl Polym Sci, 2010" @default.
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- W2151486750 date "2010-01-01" @default.
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- W2151486750 title "Diffusion coefficients of polychlorinated biphenyls and polycyclic aromatic hydrocarbons in polydimethylsiloxane and low-density polyethylene polymers" @default.
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- W2151486750 doi "https://doi.org/10.1002/app.31704" @default.
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