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- W2151504277 abstract "Ag(I)/ZSM-5 catalyst was prepared and characterized spectroscopically in relation to its photocatalytic reactivity for the photodecomposition of nitric oxide. UV irradiation of the Ag(I)/ZSM-5 catalyst in the presence of NO leads to efficient catalytic conversion of NO into N2, O2, and other nitrogen oxides. Emission and synchronous-scan photoluminescence spectra indicate the presence of several environments for the Ag(I) ions in the ZSM-5 host. Ground- and excited-state electronic structure calculations for models in which [Ag+]n ions (n ≥ 1) are coordinated to NO molecules, suggest that N−O bonds are stronger in the ground state while N−N and O−O bonds are stronger in certain excited states. The luminescence and molecular orbital data suggest that more than one catalytic site for the photodecomposition of NO is present in Ag(I)/ZSM-5. The results of EXAFS have been used in support of the excited-state assignments." @default.
- W2151504277 created "2016-06-24" @default.
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- W2151504277 date "2000-03-29" @default.
- W2151504277 modified "2023-10-17" @default.
- W2151504277 title "Characterization of the Excited States Responsible for the Action of Silver(I)-Doped ZSM-5 Zeolites as Photocatalysts for Nitric Oxide Decomposition" @default.
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- W2151504277 doi "https://doi.org/10.1021/jp992703c" @default.
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