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- W2153833408 abstract "The cyclic voltammetry of the reductive cleavage of N-fluoro-, N-chloro-, and N-bromosaccharin sultams and of their 4-nitro-substituted analogues was investigated in acetonitrile at an inert electrode. The seriin of compounds provides particularly clear evidence that the two main factors governing the occurrence of a stepwise or a concerted mechanism in reductive cleavages are the energy of the π * orbital, possibly accommodating the incoming electron, and the strength of the breaking bond. In the concerted cases, application of the theory of dissociative electron transfer allowed the intimation of the nitrogen-halogen bond dissociation energy and of the standard potential and intrinsic barrier of the reaction" @default.
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- W2153833408 date "2010-08-20" @default.
- W2153833408 modified "2023-09-30" @default.
- W2153833408 title "ChemInform Abstract: Controlling Factors of Stepwise Versus Concerted Reductive Cleavages. Illustrative Examples in the Electrochemical Reductive Breaking of Nitrogen-Halogen Bonds in Aromatic N-Halosultams." @default.
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- W2153833408 doi "https://doi.org/10.1002/chin.199347049" @default.
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