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- W2153874383 abstract "A new donor–acceptor system, in which the electron donor triphenylamine (TPA) and the electron acceptor C60 are bridged through a cis- or trans-platinum(II) acetylide spacer have been prepared. Ground-state studies were conducted using electrochemistry and UV/Vis spectroscopy. Fluorescence studies suggested that charge transfer is the deactivation mechanism for the singlet excited state, and this was verified by transient absorption spectroscopy. Selective photoexcitation of 1 and 2 at 387 nm leads to a fast charge transfer between the TPA and C60, which gives rise to a radical ion-pair state (TPA.+–Pt–C60.−). Our results suggest that charge transfer is favored for the cis configuration while the presence of the trans configuration in the PtII diacetylide results in a longer-lived charge separated states." @default.
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- W2153874383 date "2014-07-30" @default.
- W2153874383 modified "2023-10-11" @default.
- W2153874383 title "Geometric Influence on Intramolecular Photoinduced Electron Transfer in Platinum(II) Acetylide-Linked Donor-Acceptor Assemblies" @default.
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- W2153874383 doi "https://doi.org/10.1002/chem.201402616" @default.
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- W2153874383 hasPublicationYear "2014" @default.
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