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- W2154013453 abstract "Thorough understanding of H2 electrochemical oxidation helps optimize SOFC anode design and improve its performance. However, controversies still exist regarding H2 electrochemical oxidation. Due to their well-defined 2-D structure, Ni/YSZ pattern anodes are ideally suited for reaction kinetic studies. In this study, a systematic study was performed to determine conditions for the stabilization of Ni/YSZ pattern anode performance. Moreover, a comprehensive and reliable dataset of H2 electrochemical oxidation was obtained under stable test conditions. We found that stabilization of Ni/YSZ pattern anode performance relies on temperature and Ni thickness. Polarization resistance (Rp) depends on temperature, overpotential, H2 partial pressure, and TPB length, and it increases with decreasing any of these parameters. Rp also depends on H2O content. When the pH2O is between 3000 Pa (3 % of the total gases) and 30 000–40 000 Pa (30–40 % of the total gases), Rp decreases with increasing H2O content. However, Rp is less affected with further increasing H2O content. Charge transfer reactions coupled with H2O-related processes contribute to the rate-limiting steps for H2 electro-oxidation." @default.
- W2154013453 created "2016-06-24" @default.
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- W2154013453 date "2015-10-07" @default.
- W2154013453 modified "2023-09-24" @default.
- W2154013453 title "Stability and electrochemical performance of Ni/YSZ pattern anodes in H<sub>2</sub>/H<sub>2</sub>O atmosphere" @default.
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- W2154013453 doi "https://doi.org/10.1002/cjce.22330" @default.
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