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- W2154373214 abstract "Abstract Time‐resolved and product studies on the synthesized dyads 1 and 2 have provided evidence that the benzophenone‐to‐thymine orientation strongly influences intramolecular photophysical and photochemical processes. The prevailing reaction mechanism has been established as a Paterno–Büchi cycloaddition to give oxetanes 3 – 6 ; however, the ability of benzophenone to achieve a formal hydrogen abstraction from the methyl group of thymidine has also been evidenced by the formation of photoproducts 7 and 8 . These processes have been observed only in the case of the cisoid dyad 1 . Adiabatic photochemical cycloreversion of the oxetane ring is achieved upon direct photolysis to give the starting dyad 1 in its excited triplet state. The photobiological implications of the above results are discussed with respect to benzophenone‐photosensitized damage of thymidine." @default.
- W2154373214 created "2016-06-24" @default.
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- W2154373214 date "2005-12-19" @default.
- W2154373214 modified "2023-10-17" @default.
- W2154373214 title "Intramolecular Interactions in the Triplet Excited States of Benzophenone–Thymine Dyads" @default.
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- W2154373214 doi "https://doi.org/10.1002/chem.200500345" @default.
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