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• W2155079462 abstract "The emission spectrum of VCl has been investigated at high resolution in the 3000–19 400 cm−1 region using a Fourier transform spectrometer. The bands were excited in a high temperature carbon tube furnace by the reaction of vanadium metal vapor and a trace of BCl3 as well as in a microwave discharge lamp by the reaction of VOCl3 vapor with active nitrogen. The spectra were recorded using the Fourier transform spectrometer associated with the McMath–Pierce telescope of the National Solar Observatory at Kitt Peak. The analysis of the E5Δ–X5Δ system of VCl (previously labeled as [7.0]5Δ–X5Δ) has been extended by analyzing the rotational structure of some additional bands. A rotational analysis of the 5Δ1–5Δ1, 5Δ3–5Δ3, and 5Δ4–5Δ4 subbands of the 0–2, 0–1, 0–0, and 1–0 bands, and the 5Δ2−5Δ2 subband of the 0–1 and 0–0 bands has been obtained and molecular constants have been extracted. The 5Δ0±−5Δ0± subband was not identified in any of the assigned bands. The spectroscopic properties of the low-lying electronic states of VCl have been predicted by CASSCF/CMRCI ab initio calculations and the experimental assignments are supported by the ab initio results." @default.
• W2155079462 created "2016-06-24" @default.
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• W2155079462 date "2003-02-01" @default.
• W2155079462 modified "2023-09-27" @default.
• W2155079462 title "Infrared emission spectroscopy and ab initio calculations on VCl" @default.
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• W2155079462 doi "https://doi.org/10.1016/s0022-2852(02)00016-4" @default.
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