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• W2155644807 abstract "A picosecond pump and probe experiment has been applied to study the excited state dynamics of 7-azaindole-water 1 ∶ 2 and 1 ∶ 3 clusters [7AI(H(2)O)(2,3)] in the gas phase. The vibrational-mode selective Excited-State-Triple-Proton Transfer (ESTPT) in 7AI(H(2)O)(2) proposed from the frequency-resolved study has been confirmed by picosecond decays. The decay times for the vibronic states involving the ESTPT promoting mode σ(1) (850-1000 ps) are much shorter than those for the other vibronic states (2100-4600 ps). In the (1 + 1) REMPI spectrum of 7AI(H(2)O)(3) measured by nanosecond laser pulses, the vibronic bands with an energy higher than 200 cm(-1) above the origin of the S(1) state become very weak. In contrast, the vibronic bands in the same region emerge in the (1 + 1') REMPI spectrum of 7AI(H(2)O)(3) with picosecond pulses. The decay times drastically decrease when increasing the vibrational energy above 200 cm(-1). Ab initio calculations show that a second stable cyclic-nonplanar isomer exists in addition to a bridged-planar isomer, and that an isomerization from a bridged-planar isomer to a cyclic-nonplanar isomer is most probably responsible for the short lifetimes of the vibronic states of 7AI(H(2)O)(3)." @default.
• W2155644807 created "2016-06-24" @default.
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• W2155644807 date "2011-01-01" @default.
• W2155644807 modified "2023-10-16" @default.
• W2155644807 title "Photon induced isomerization in the first excited state of the 7-azaindole–(H2O)3 cluster" @default.
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• W2155644807 doi "https://doi.org/10.1039/c1cp00015b" @default.
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