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- W2155724668 abstract "Four new manganese(III) porphyrins, heterogenised as insoluble zinc phosphonates, exhibit behaviour markedly different from their homogeneous counterparts in the competitive hydroxylation of alkane mixtures (i.e., cyclododecane–cyclohexane), using iodosylbenzene as the oxidant. The cyclohexanol:cyclododecanol ratio can be increased by as much as five, owing to shape selectivity effects imposed by the phosphonate support. Se′lectivite′ de forme pour l'hydroxylation d'alcanes, catalyse′e par des porphyrines de manganese he′te′roge′ne′ise′es sous forme de phosphonates de zinc. Une se′rie de quatre te′traarylporphyrines de manganese(III) he′te′roge′ne′ise′es sous forme de phosphonates de zinc insolubles, teste′es pour l'hyroxylation compe′titive de me′langes d'alcanes (par exemple, cyclodode′cane–cyclohexane) par l'iodosobenzene, montrent un comportement tres diffe′rent de celui de leurs homologues non supporte′s en milieu homogene. Le rapport cyclohexanol:cyclodode′canol peut augmenter d'un facteur allant jusqu'a cinq, sous l'effet d'une se′lectivite′ de forme induite par le support phosphonate." @default.
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- W2155724668 date "1998-01-01" @default.
- W2155724668 modified "2023-09-27" @default.
- W2155724668 title "Shape selectivity for alkane hydroxylation with a new class of phosphonate-based heterogenised manganese porphyrins" @default.
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