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• W2156883061 endingPage "9532" @default.
• W2156883061 startingPage "9528" @default.
• W2156883061 abstract "The first Ni(0)/bis(oxazoline)-catalyzed asymmetric denitrogenative transannulation of 1,2,3-benzotriazin-4(3H)-ones with bulky internal alkynes to form novel axially chiral isoquinolones in an atroposelective manner has been developed. This method provides direct asymmetric access to axially chiral isoquinolones with excellent functional-group tolerance in excellent yields and stereoselectivities from readily available starting materials under mild reaction conditions. These axially chiral isoquinolones exhibit high cytotoxicity against a number of human cancer cell lines. DFT calculations reveal the nature of the transition state in the key annulation step." @default.
• W2156883061 created "2016-06-24" @default.
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• W2156883061 date "2015-06-26" @default.
• W2156883061 modified "2023-10-16" @default.
• W2156883061 title "Asymmetric Synthesis of Axially Chiral Isoquinolones: Nickel-Catalyzed Denitrogenative Transannulation" @default.
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• W2156883061 doi "https://doi.org/10.1002/anie.201503207" @default.
• W2156883061 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/26119725" @default.
• W2156883061 hasPublicationYear "2015" @default.
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