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• W2157256008 abstract "Abstract The surface areas and uptake of CO 2 and CH 4 by four graphene samples are measured and compared with activated charcoal. The surface areas are in the range of 5–640 m 2 g −1 , whereas the CO 2 and CH 4 uptake values are in the range of 18–45 wt % (at 195 K, 0.1 MPa) and 0–2.8 wt % (at 273 K, 5 MPa), respectively. The CO 2 and CH 4 uptake values of the graphene samples vary linearly with the surface area. In contrast, graphene‐like B x C y N z samples with compositions close to BC 2 N exhibit surface areas in the range of 1500–1990 m 2 g −1 and CO 2 and CH 4 uptake values in the ranges 97–128 wt % (at 195 K, 0.1 MPa) and 7.5–17.3 wt %, respectively. The uptake of these gases varies exponentially with the surface area of the B x C y Z n samples, and the uptake of CH 4 varies proportionally with that of CO 2 . The uptake of CO 2 for the best BC 2 N sample is 64 wt % at 298 K. The large uptake of both CO 2 and CH 4 gases by BC 2 N betters the performance of graphenes and activated charcoal. First‐principles calculations show that the adsorption of CO 2 and CH 4 is more favored on BCN samples compared to graphene." @default.
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• W2157256008 date "2011-08-25" @default.
• W2157256008 modified "2023-10-18" @default.
• W2157256008 title "Remarkable Uptake of CO2 and CH4 by Graphene-Like Borocarbonitrides, BxCyNz" @default.
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• W2157256008 doi "https://doi.org/10.1002/cssc.201100197" @default.
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