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• W2157294920 abstract "Most recently, much attention has been devoted to 1T phase MoS2 because of its distinctive phase-engineering nature and promising applications in catalysts, electronics, and energy storage devices. While alkali metal intercalation and exfoliation methods have been well developed to realize unstable 1T-MoS2 , but the aqueous synthesis for producing stable metallic phase remains big challenging. Herein, a new synthetic protocol is developed to mass-produce colloidal metallic 1T-MoS2 layers highly stabilized by intercalated ammonium ions (abbreviated as N-MoS2). In combination with density functional calculations, the X-ray diffraction pattern and Raman spectra elucidate the excellent stability of metallic phase. As clearly depicted by high-angle annular dark-field imaging in an aberration-corrected scanning transmission electron microscope and extended X-ray absorption fine structure, the N-MoS2 exhibits a distorted octahedral structure with a 2a0 × a0 basal plane superlattice and 2.72 Å Mo-Mo bond length. In a proof-of-concept demonstration for the obtained material's applications, highly efficient photocatalytic activity is achieved by simply hybridizing metallic N-MoS2 with semiconducting CdS nanorods due to the synergistic effect. As a direct outcome, this CdS:N-MoS2 hybrid shows giant enhancement of hydrogen evolution rate, which is almost 21-fold higher than pure CdS and threefold higher than corresponding annealed CdS:2H-MoS2." @default.
• W2157294920 created "2016-06-24" @default.
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• W2157294920 date "2015-08-31" @default.
• W2157294920 modified "2023-10-18" @default.
• W2157294920 title "Gram-Scale Aqueous Synthesis of Stable Few-Layered 1T-MoS₂: Applications for Visible-Light-Driven Photocatalytic Hydrogen Evolution" @default.
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• W2157294920 doi "https://doi.org/10.1002/smll.201501822" @default.
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• W2157294920 hasPublicationYear "2015" @default.
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