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- W2157356211 abstract "The presence of mesopores in the interior of microporous particles may significantly improve their transport properties. Complementing previous macroscopic transient sorption experiments and pulsed field gradient NMR self-diffusion studies with such materials, the present study is dedicated to an in-depth study of molecular uptake and release on the individual particles of mesoporous zeolitic specimens, notably with samples of the narrow-pore structure types, CHA and LTA. The investigations are focused on determining the time constants and functional dependences of uptake and release. They include a systematic variation of the architecture of the mesopores and of the guest molecules under study as well as a comparison of transient uptake with blocked and un-blocked mesopores. In addition to accelerating intracrystalline mass transfer, transport enhancement by mesopores is found to be, possibly, also caused by a reduction of transport resistances on the particle surfaces." @default.
- W2157356211 created "2016-06-24" @default.
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- W2157356211 date "2013-07-04" @default.
- W2157356211 modified "2023-10-16" @default.
- W2157356211 title "Diffusion Study by IR Micro-Imaging of Molecular Uptake and Release on Mesoporous Zeolites of Structure Type CHA and LTA" @default.
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- W2157356211 doi "https://doi.org/10.3390/ma6072662" @default.
- W2157356211 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5521224" @default.
- W2157356211 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/28811401" @default.
- W2157356211 hasPublicationYear "2013" @default.
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