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• W2157503804 abstract "We have investigated the fracture behaviors of tetra-arm polyethylene glycol (Tetra-PEG) gels with controlled network structures. Tetra-PEG gels were prepared by AB-type crosslink-coupling of mutually reactive tetra-arm prepolymers with different concentrations and molecular weights. This series of controlled network structures, for the first time, enabled us to quantitatively examine the Lake-Thomas model, which is the most popular model predicting fracture energies of elastomers. The experimental data showed good agreement with the Lake-Thomas model, and indicated a new molecular interpretation for the displacement length (L), the area around a crack tip within which the network strands are fully stretched. L corresponded to the three times of end-to-end distance of network strands, regardless of all parameters examined. We conclude that the Lake-Thomas model can quantitatively predict the fracture energy of polymer network without trapped entanglements, with the enhancement factor being near 3." @default.
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• W2157503804 date "2013-10-11" @default.
• W2157503804 modified "2023-10-02" @default.
• W2157503804 title "Fracture energy of polymer gels with controlled network structures" @default.
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• W2157503804 doi "https://doi.org/10.1063/1.4823834" @default.
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• W2157503804 hasPublicationYear "2013" @default.
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