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• W2157777502 abstract "The answers to the question posed in the title are different for the two compounds: In the case of 1 the X-ray crystal structure observed at 100 K is that corresponding to the transition state of the free molecule between the two possible valence tautomers. In contrast, the crystal of 2 contains molecules with rectangular arrangement of the four-membered ring in two orientations rotated through 90°. The transition state of 1 in the crystal is the energetically more favored state since it enables a better packing of the tert-butyl groups. These investigations disprove afresh the nearly square arrangement considered as plausible for the four-membered ring atoms of 2 on steric grounds." @default.
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• W2157777502 date "1988-03-01" @default.
• W2157777502 modified "2023-10-17" @default.
• W2157777502 title "Equilibrium Structure, Stabilized Transition State, or Disorder in the Crystal? Studies of the Antiaromatic Systems Tetra-<i>tert</i>-butyl-<i>s</i>-indacene and Tetra-<i>tert</i>-butylcyclobutadiene by Low-Temperature Crystal Structure Analysis" @default.
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• W2157777502 doi "https://doi.org/10.1002/anie.198803871" @default.
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