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- W2159214724 abstract "The purpose of this study was to elucidate the processes controlling the distribution and behavior of the longerlived Ra isotopes in continuous Paleozoic carbonate aquifers of parts of Missouri, Kansas, and Oklahoma. Activities of ( 228 Ra) and ( 226 Ra) were analyzed in fresh and saline ground waters, brines, and rocks. The fluids have a wide salinity range (200‐250,000 mg l ˇ1 total dissolved solids). The ( 226 Ra) activity ranges from 0.66‐7660 dpm kg ˇ1 and correlates with salinity and other alkaline earth element (Ca, Sr, and Ba) concentrations. The range of ( 228 Ra: 226 Ra) ratios in the fluids (0.06‐1.48) is similar to that in the aquifer rocks (0.21‐1.53). The relatively low mean fluid ( 228 Ra: 226 Ra) ratio (0.30) reflects the low Th:U ratio of the predominant carbonate aquifer rock. Radium occurs mostly (r77%) as Ra 2+ species in the fluids. Salinity-dependent sorption‐desorption processes (with log K values from 10 0 ‐10 4 and negatively correlated with salinity), involving Th-enriched surface coatings on aquifer flow channels, can explain the rapid solid‐fluid transfer of Ra isotopes in the system and the correlation of Ra with" @default.
- W2159214724 created "2016-06-24" @default.
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- W2159214724 date "2001-01-01" @default.
- W2159214724 modified "2023-10-10" @default.
- W2159214724 title "Radium geochemistry of ground waters in Paleozoic carbonate aquifers, midcontinent, USA" @default.
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- W2159214724 doi "https://doi.org/10.1016/s0883-2927(00)00014-7" @default.
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