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• W2160485335 abstract "The infrared spectrum of the AsD3 molecule has been measured in the region of the stretching fundamental bands on a Fourier transform spectrometer with a resolution of 0.0027 cm−1 and analyzed for the first time. More than 3300 normally allowed and in addition more than 900 forbidden, but perturbation-allowed transitions with Jmaxupper=28 have been assigned to the bands ν1 and ν3. An effective Hamiltonian was used which takes into account the resonance interactions between the states (1000) and (0010). A set of 50 (26 diagonal and 24 resonance) refined spectroscopic parameters was obtained from the fit which reproduces the 1229 initial ‘experimental’ upper state ro-vibrational energies with an rms deviation of 0.00024 cm−1. The transition moment ratio |μ1:μ3| was determined to be 1.2±0.05, and the intensity perturbation μ1 ξ13y μ3 found to be negative. The equilibrium values of the bond length rAs–De=1.51130(11)Å and interbond angle αD–As–De=92.0775(40)˚ were determined from the values of the rotational parameters of the ground state and the four fundamental bands." @default.
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• W2160485335 date "2006-01-01" @default.
• W2160485335 modified "2023-09-26" @default.
• W2160485335 title "High-resolution infrared study of the ν1 and ν3 bands, and the equilibrium structure of AsD3" @default.
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• W2160485335 doi "https://doi.org/10.1016/j.molstruc.2005.05.054" @default.
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