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- W2160642610 abstract "Electrochemical CO 2 reduction was studied by using a graphite electrode coated with cobalt octacyanophthalocyanine ( CoPc ( CN ) 8 ) and dipped in an aqueous phase. The most active and selective CO 2 reduction was achieved at −1.20 V (vs Ag / AgCl ) with the ratio of the produced CO / H 2 around 10 at pH 9.3. The electrocatalytic CO 2 reduction by CoPc ( CN ) 8 could be achieved at a more positive applied potential than non-substituted CoPc ( CoPc ), which can be ascribed to the relatively positive redox potential of CoPc ( CN ) 8 . The catalytic mechanism of the CoPc ( CN ) 8 in a homogeneous system was investigated by an in situ potential-step chronoamperospectroscopy under argon and under CO 2 as well. In CoPc ( CN ) 8 the rate-determining step was an intermediate formation step, while in CoPc it was the second reduction of the complex." @default.
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- W2160642610 date "1997-10-01" @default.
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- W2160642610 title "Electrochemical <font>CO</font><sub>2</sub> Reduction Catalysed by Cobalt Octacyanophthalocyanine and its Mechanism" @default.
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- W2160642610 doi "https://doi.org/10.1002/(sici)1099-1409(199710)1:4<315::aid-jpp35>3.0.co;2-v" @default.
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