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- W2162096298 abstract "The synthesis of a new soluble conjugated porphyrin polymer 4 is reported. The MALDI TOF mass spectrum shows the presence of oligomers with up to 13 repeat units and GPC gives a Mn of 53 kDa. The electronic absorption spectra of this polymer exhibit an intense Q band at 800 nm in solution and 853 nm in the solid state, demonstrating a high degree of conjugation. Electroabsorption spectroscopy shows that thin films of 4 have lower resonant third order NLO susceptibility than our previous conjugated porphyrin polymer 2, whereas closed z-scan measurements indicate that the off-resonance real susceptibility, at 1064 nm, is exceptionally large for both polymers (χ(3)R = −2 × 10−16 m2 V−2). Open z-scan measurements were also made at 1064 nm, demonstrating that the two polymers exhibit similar nonlinear absorption at this wavelength (β = 1 cm GW−1 at 0.2 mM concentration)." @default.
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- W2162096298 date "2001-01-01" @default.
- W2162096298 modified "2023-10-14" @default.
- W2162096298 title "Synthesis and third order nonlinear optics of a new soluble conjugated porphyrin polymer" @default.
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- W2162096298 doi "https://doi.org/10.1039/b007250h" @default.
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