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- W2162224440 abstract "Fuel synthesis through coal and biomass gasification can potentially provide a solution to the increasing demand of energy and transportation fuels. To theoretically understand the complex chemical processes in a gasifier and to identify the most influential parameters on syngas production, a multi-scale model with detailed chemistry was developed for the first time to simulate the gasification processes in a well-stirred reactor. The model considers gasphase and particle-phase reactions as well as coupling between the two phases at various scales (mass and energy exchange). The gas-phase reactions use the detailed chemistry GRIMech 1.2 including 177 elementary reactions and 31 species as well as multi-component transport properties and variable thermodynamic properties. For the particle-phase, four surface reactions were considered (C+O2=CO2, C+H2O=CO+H2, C+CO2=2CO, C+2H2=CH4). And the reaction rates were simulated by the diffusion-kinetic model with consideration of boundary layer diffusion. The coupling between the two phases including exchange of mass and energy were modeled. A code was developed to solve gas-phase and particle-phase governing equations. Numerical simulations were conducted to understand the gasification process and the effects of pressure, O2 concentration and H2 addition on gasification performance." @default.
- W2162224440 created "2016-06-24" @default.
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- W2162224440 date "2011-01-04" @default.
- W2162224440 modified "2023-09-24" @default.
- W2162224440 title "Multi-scale Modeling of Coal Gasification Processes in a Well-Stirred Reactor with Detailed Chemistry" @default.
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- W2162224440 doi "https://doi.org/10.2514/6.2011-116" @default.
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