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- W2162269673 abstract "Abstract The standard Gibbs free energies of formation of Sr2RhO4(s) and Sr4RhO6(s) have been determined using two types of solid-state electrochemical cells: one using CaF2(s) as the solid electrolyte, the fluoride cell and the other wherein calcia-stabilized zirconia (CSZ) has been used as the solid electrolyte, the oxide cell. The fluoride cell was operated in the temperature range from 895 to 1018 K and can be represented by (−) Pt / O 2 ( g ),{ CaO ( s )+ CaF 2 ( s )}// CaF 2 //{ SrF 2 ( s )+ Sr 2 RhO 4 ( s )+ Sr 4 RhO 6 ( s )} O 2 ( g )/ Pt (+) and the oxide cell was operated in the temperature range from 1092 to 1267 K and can be represented by (−) Pt /{ Sr 2 RhO 4 ( s )+ Sr 4 RhO 6 ( s )+ Rh ( s )}// CSZ // O 2 (p( O 2 )=21.21 kPa )/ Pt (+) The standard Gibbs free energies of formation of Sr2RhO4(s) and Sr4RhO6(s) from elements in their standard state, calculated by combining results obtained from fluoride and oxide cells, can be given respectively by Δ f G°{ Sr 2 RhO 4 ( s )}( kJ mol −1 )(±2)=−1617.7+0.4998 (T), Δ f G°{ Sr 4 RhO 6 ( s )}( kJ mol −1 )(±2)=−2947.1+0.8284 (T) ." @default.
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- W2162269673 date "2004-11-01" @default.
- W2162269673 modified "2023-09-27" @default.
- W2162269673 title "Simultaneous determination of Gibbs free energies of formation of Sr2RhO4(s) and Sr4RhO6(s) using solid-state electrochemical cells" @default.
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- W2162269673 doi "https://doi.org/10.1016/j.jallcom.2004.03.105" @default.
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