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- W2164485303 abstract "A numerical model has been developed to predict the local concentrations of chemical species throughout the anolyte compartment in a simplified chlor-alkali reactor with a flow channel defined by a pair of parallel-plate electrodes. Mass transport by diffusion, migration, and advection has been approximated by numerically solving the Nernst-Planck equation for each species, coupled with a set of nonlinear and linear algebraic equations describing the chemistry and electroneutrality. The predicted concentration profiles for protons, chloride ions, chlorine, and hypochlorous acid/hypochlorite ions exhibit large concentration changes in the membrane boundary layer. The sharp pH increase from a bulk value of 2 to ca. 6 at the membrane would allow the undesirable local decomposition of hypochlorite to chlorate ions, which are produced in industrial reactors." @default.
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- W2164485303 date "2000-01-01" @default.
- W2164485303 modified "2023-09-24" @default.
- W2164485303 title "Numerical Modeling of the Mass Transport and Chemistry of a Simplified Membrane-Divided Chlor-Alkali Reactor" @default.
- W2164485303 doi "https://doi.org/10.1149/1.1394037" @default.
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