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• W2165368889 abstract "Thin films of the type I clathrate Ba <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>8</sub> Ga <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>16</sub> Ge <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>30</sub> have been synthesized by the pulsed laser ablation technique. The relatively low ablation threshold of this material at the UV wavelength leads to the ejection of particulates during laser-target interaction. The optimum laser fluence for the formation of stoichiometric films with the lowest particle density was 2.5 J/cm <sup xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2 </sup> . Excitation of the UV laser generated plasma by a second pulsed CO <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>2</sub> laser further reduced particulate ejection and produced broader expansion profiles leading to large area uniform films. Films deposited by this method on quartz substrates were polycrystalline and showed semiconducting behavior. High purity type II Na <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>x</sub> Si <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>136</sub> clathrates in bulk form have been synthesized by solid state reactions. The electrical properties of Na <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>x</sub> Si <sub xmlns:mml=http://www.w3.org/1998/Math/MathML xmlns:xlink=http://www.w3.org/1999/xlink>136</sub> (0 < x < 24) clathrates show a clear dependence on Na content, with resistivities that span several orders of magnitude" @default.
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• W2165368889 date "2006-01-01" @default.
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• W2165368889 title "Synthesis and Characterization of Bulk and Thin Film Clathrates for Solid State Power Conversion Applications" @default.
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• W2165368889 doi "https://doi.org/10.1109/ict.2006.331266" @default.
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