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• W2165802023 abstract "We extend previous studies of the dynamical relaxation in liquids consisting of particles interacting with the soft-sphere or inverse power potential, , where e and σ set the energy and length scales, respectively, and n is the steepness or stiffness parameter. In previous work we have simulated these systems using molecular dynamics (MD) simulation. Here we include model colloidal particles interacting with this potential, executing the position Langevin equation of motion as implemented in the Brownian dynamics (BD), method. A formal statistical mechanical expansion of the force autocorrelation function for such particles was carried out in both cases. Using the (molecular) Liouville operator this gives at short time a scaling with time, t, in terms of a reduced time, , where d depends on the state point, and for the colloidal case, the Smoluchowski operator gives the reduced time, . The first term accounts for the leading two-body contributions to the relaxation, and the second term, in d, represents a..." @default.
• W2165802023 created "2016-06-24" @default.
• W2165802023 creator A5027973161 @default.
• W2165802023 creator A5036654343 @default.
• W2165802023 date "2005-09-10" @default.
• W2165802023 modified "2023-09-27" @default.
• W2165802023 title "The effects of particle softness on the dynamics of molecular and colloidal systems" @default.
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• W2165802023 doi "https://doi.org/10.1080/00268970500105029" @default.
• W2165802023 hasPublicationYear "2005" @default.
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