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• W2166337315 abstract "The calculation of the external work expended during the switching between two systems yields bounds on their free energy difference. The quality of these bounds depends on the choice of path along which the work is calculated. In this paper, it is shown that for sufficiently fast relaxations the optimal path will be characterized by a minimal thermodynamic length, and that it should be parametrized such that it is traversed with constant thermodynamic speed. As an example, the optimal switching of a magnetic field containing a paramagnet is considered. Finally, the effects of finite relaxation times are discussed." @default.
• W2166337315 created "2016-06-24" @default.
• W2166337315 creator A5043858152 @default.
• W2166337315 date "1996-12-08" @default.
• W2166337315 modified "2023-10-16" @default.
• W2166337315 title "A thermodynamic distance criterion of optimality for the calculation of free energy changes from computer simulations" @default.
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• W2166337315 doi "https://doi.org/10.1063/1.472836" @default.
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