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- W2166805782 abstract "Monomolecular fragmentations of butadiyne- and 1,3-pentadiyne radical cations in their electronically excited states have been investigated by use of the photoelectron-photoion coincidence technique. Breakdown curves for the molecular and various fragment ions have been recorded over the ionization energy range of 9 to 17 eV. These breakdown curves reveal the extent of the competition between the radiative relaxation (ion fluorescence) and the non-radiative internal conversion followed by fragmentation for the decay of the first excited electronic states. Extensive hydrogen scrambling and/or ionic-carbon-skeleton isomerization takes place prior to fragmentation, as revealed by the breakdown curves obtained for the site specifically deuteriated 1,3-pentadiynes." @default.
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- W2166805782 date "1979-10-31" @default.
- W2166805782 modified "2023-10-03" @default.
- W2166805782 title "Fragmentation of Energy Selected Butadiyne- and 1,3-Pentadiyne Radical Cations" @default.
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- W2166805782 doi "https://doi.org/10.1002/hlca.19790620716" @default.
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