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- W2166846240 abstract "Abstract The now 20-year old experiments of and Kovacs on the volumetric recovery of poly(viny1 acetate) near its glass transition brought to light several unexpected results: although the kinetics of recovery of the equilibrium volume following a downward step in temperature seemed describable by a free volume model, the recovery kinetics following an upward step in temperature clearly was not a function of free volume alone. In other experiments involving a pair of temperature steps, in which the pair of steps and the time interval between was programmed to bring the glass to an equilibrium volume at the instant the second temperature step was made, the volume following the second step drifted away from this equilibrium value and then returned to it later. Although Kovacs, Aklunis, and Hutchinson have shown recently that these early results could be described by a linear irreversible thermodynamic theory with a set of 33 ordering parameters, we believe the molecular origin of these results is fairly sim..." @default.
- W2166846240 created "2016-06-24" @default.
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- W2166846240 date "1980-01-01" @default.
- W2166846240 modified "2023-09-24" @default.
- W2166846240 title "Local motion, free volume fluctuations, and the thermodynamic recovery of polymeric glasses" @default.
- W2166846240 doi "https://doi.org/10.1080/00222348008241856" @default.
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