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- W2169294562 abstract "The synthesis of a carbazole-derived, well-defined ladder polymer was achieved under thermodynamic control by employing reversible ring-closing olefin metathesis. This unique approach featured mild conditions and excellent efficiency, affording the ladder polymer backbone with minimum levels of unreacted defects. Rigorous NMR analysis on a 13C isotope-enriched product revealed that the main-chain contained less than 1% of unreacted precursory vinyl groups. The rigid conformation of the ladder-type backbone was confirmed by photophysical analysis, while the extended rod-like structure was visualized under scanning tunneling microscope. Excellent solubility of this polymer in common organic solvents allowed for feasible processing of thin films using solution-casting techniques. Atomic force microscopy and grazing incident X-ray scattering revealed a uniform and amorphous morphology of these films, in sharp contrast to the polycrystalline thin films of its small molecular counterpart." @default.
- W2169294562 created "2016-06-24" @default.
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- W2169294562 date "2016-01-01" @default.
- W2169294562 modified "2023-09-30" @default.
- W2169294562 title "Thermodynamic synthesis of solution processable ladder polymers" @default.
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- W2169294562 doi "https://doi.org/10.1039/c5sc02385h" @default.
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