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- W2169304278 abstract "The homogeneous gas-phase reaction CH3COSH + CH2:CO ⇆ Ac2S has been studied in both directions over the temperature range 128–253°. The forward reaction is of the second order, k= 105·45 exp (–37,900/RT) l mol–1 s–1, and the back reaction first order, k= 1011·02 exp (–131,000/RT) s–1. Equilibrium constants were measured starting from both sides of the reaction, and calculated from the ratio of the rate constants. From the mean of these was obtained ΔH°=–94·7 kJ mol–1 and ΔS°=–140·8 J K–1 mol–1. Results are compared with those obtained for the keten–acetic acid system." @default.
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- W2169304278 date "1974-01-01" @default.
- W2169304278 modified "2023-09-24" @default.
- W2169304278 title "Reactions of keten. Part IV. Kinetics and thermodynamics of the gas-phase reaction: thioacetic acid + keten ? acetic thioanhydride" @default.
- W2169304278 doi "https://doi.org/10.1039/p29740001879" @default.
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