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- W2169478440 abstract "A series of electronically dissymmetric all-organic macrocycles were synthesized using straightforward synthetic procedures. These macrocycles vary in the nature of the substituents, the geometry of the linkage that connects the electron-deficient aromatic ring, the type of linkage, and the presence or absence of a heteroaromatic ring. These small structural variations impart significant differences in the performance of these macrocycles in binding benzo[a]pyrene, with binding constants up to 2.5 × 104 M–1 obtained. They also lead to significant differences in their ability to promote non-covalent energy transfer from benzo[a]pyrene to a BODIPY fluorophore, with energy transfer efficiencies ranging from 32 % to 398 %. These differences can be explained using a variety of computational investigative techniques, which highlight the flexibility of the macrocycle architectures to accommodate benzo[a]pyrene and to promote close donor–acceptor interactions." @default.
- W2169478440 created "2016-06-24" @default.
- W2169478440 creator A5027066179 @default.
- W2169478440 creator A5091513628 @default.
- W2169478440 date "2015-08-12" @default.
- W2169478440 modified "2023-10-18" @default.
- W2169478440 title "Rationally Designed Supramolecular Organic Hosts for Benzo[<i>a</i>]pyrene Binding and Detection" @default.
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- W2169478440 doi "https://doi.org/10.1002/ejoc.201500684" @default.
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