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• W2169769897 abstract "This paper describes a systematic study on the epitaxial overgrowth of Pt on well-defined Pd nanocrystals with different shapes (and exposed facets), including regular octahedrons, truncated octahedrons, and cubes. Two different reducing agents, i.e., citric acid and L-ascorbic acid, were evaluated and compared for the reduction of K2PtCl4 in an aqueous solution in the presence of Pd nanocrystal seeds. When citric acid was used as a reducing agent, conformal overgrowth of octahedral Pt shells on regular and truncated octahedrons of Pd led to the formation of Pd-Pt core-shell octahedrons, while non-conformal overgrowth of Pt on cubic Pd seeds resulted in the formation of an incomplete octahedral Pt shell. On the contrary, localized overgrowth of Pt branches was observed when L-ascorbic acid was used as a reducing agent regardless of the facets expressed on the surface of Pd nanocrystal seeds. This work shows that both the binding affinity of a reducing agent to the Pt surface and the reduction kinetics for a Pt precursor play important roles in determining the mode of Pt overgrowth on Pd nanocrystal surface." @default.
• W2169769897 created "2016-06-24" @default.
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• W2169769897 date "2010-01-01" @default.
• W2169769897 modified "2023-10-10" @default.
• W2169769897 title "Epitaxial overgrowth of platinum on palladium nanocrystals" @default.
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• W2169769897 doi "https://doi.org/10.1039/c0nr00324g" @default.
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