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• W2170265533 endingPage "3048" @default.
• W2170265533 startingPage "3041" @default.
• W2170265533 abstract "Fluorotelomer alcohols [FTOHs, F(CF(2))(n) CH(2)CH(2)OH, n = 4, 6, and 8] are emerging environmental contaminants. Biotransformation of FTOHs by mixed bacterial cultures has been reported; however, little is known about the microorganisms responsible for the biotransformation. Here we reported biotransformation of FTOHs by two well-studied Pseudomonas strains: Pseudomonas butanovora (butane oxidizer) and Pseudomonas oleovorans (octane oxidizer). Both strains could defluorinate 4:2, 6:2, and 8:2 FTOHs, with a higher degree of defluorination for 4:2 FTOH. According to the identified metabolites, P. oleovorans transformed FTOHs via two pathways I and II. The pathway I led to the production of x:2 ketone [dominant metabolite, F(CF(2))(x)C(O)CH(3); x = n - 1, n = 6 or 8], x:2 sFTOH [F(CF(2))(x)CH(OH)CH(3)], and perfluorinated carboxylic acids (PFCAs, perfluorohexanoic, or perfluorooctanoic acid). The pathway II resulted in the formation of x:3 polyfluorinated acid [F(CF(2))(x) C(2)CH(2) COOH] and relatively minor shorter-chain PFCAs (perfluorobutyric or perfluorohexanoic acid). Conversely, P. butanovora transformed FTOHs by using the pathway I, leading to the production of x:2 ketone, x:2 sFTOH, and PFCAs. This is the first study to show that individual bacterium can bio-transform FTOHs via different or preferred transformation pathways to remove multiple --CF(2) -- groups from FTOHs to form shorter-chain PFCAs." @default.
• W2170265533 created "2016-06-24" @default.
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• W2170265533 date "2012-06-04" @default.
• W2170265533 modified "2023-10-10" @default.
• W2170265533 title "Biodefluorination and biotransformation of fluorotelomer alcohols by two alkane-degrading<i>Pseudomonas</i>strains" @default.
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• W2170265533 doi "https://doi.org/10.1002/bit.24561" @default.
• W2170265533 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/22614340" @default.
• W2170265533 hasPublicationYear "2012" @default.
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