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• W2170290436 abstract "Although pathway-specific kinetic theories are fundamentally important to describe and under- stand reversible polymerisation kinetics, they come in principle at a cost of having a large number of system-specific parameters. Here, we construct a dynamical Landau theory to describe the kinetics of activated linear supramolecular self-assembly, which drastically reduces the number of parameters and still describes most of the interesting and generic behavior of the system in hand. This phenomenological approach hinges on the fact that if nucleated, the polymerisation transition resembles a phase transition. We are able to describe hysteresis, overshooting, undershooting and the existence of a lag time before polymerisation takes o?, and pinpoint the conditions required for observing these types of phenomenon in the assembly and disassembly kinetics. We argue that the phenomenological kinetic parameter in our theory is a pathway controller, i.e., it controls the relative weights of the molecular pathways through which self-assembly takes place." @default.
• W2170290436 created "2016-06-24" @default.
• W2170290436 creator A5006256173 @default.
• W2170290436 creator A5029806652 @default.
• W2170290436 creator A5041951178 @default.
• W2170290436 date "2015-09-01" @default.
• W2170290436 modified "2023-09-25" @default.
• W2170290436 title "Dynamic Landau theory for supramolecular self-assembly" @default.
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• W2170290436 doi "https://doi.org/10.1140/epje/i2015-15105-5" @default.
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• W2170290436 hasPublicationYear "2015" @default.
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