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- W2170905482 abstract "Three-dimensional nucleation and growth on active surface sites are fundamentally important initial stages of electrodeposition of metals. Electrodeposition of Hg is a widely employed model for studies of such processes because the near-ideal hemispherical growth of its liquid nuclei can be used to check the existing theory. In this article we discuss nucleation/growth of Hg at 50–100 nm radius Pt electrodes. Recently, atomic force microscopy (AFM) was used to demonstrate that a nanoelectrode of this size has a single active site for Ag nucleation, at which the growth of a single nucleus was monitored (Chem. Sci., 2012, 3, 3307). Here we report similar observations for Hg nucleation/growth at relatively low overpotentials (e.g., 25 to 75 mV). However, at higher overpotentials (e.g., ≥100 mV), the kinetics of this process changed, and very fast multiple nucleation of Hg was observed. Possible origins of this phenomenon are discussed." @default.
- W2170905482 created "2016-06-24" @default.
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- W2170905482 date "2014-01-01" @default.
- W2170905482 modified "2023-09-27" @default.
- W2170905482 title "Nucleation and growth of mercury on Pt nanoelectrodes at different overpotentials" @default.
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- W2170905482 doi "https://doi.org/10.1039/c3sc52488d" @default.
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