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• W2171123911 endingPage "5740" @default.
• W2171123911 startingPage "5732" @default.
• W2171123911 abstract "A new family of cationic rhenium tricarbonyl complexes with either two N-alkylimidazole (N-RIm) and one pyridine (Py) ligand, or two pyridine and one N-RIm ligand, [Re(CO)3 (N-RIm)(3-x) (Py)x ](+) , has been prepared. The reaction of these complexes with a strong base, followed by an oxidant, selectively afforded 2,2'-pyridylimidazole complexes as the result of intramolecular dehydrogenative CC coupling reactions. For tris(pyridine) complexes [Re(CO)3 (Py)3 ](+) the reaction pattern upon a deprotonation/oxidation sequence is maintained, which allows the generation of complexes with 2,2'-bipyridine ligands. In the particular combination of two different types of pyridine ligand in the cationic fac-Re(CO)3 complexes only the cross-coupling products with asymmetric 2,2'-bipyridine ligands were obtained; the homocoupling products were not observed." @default.
• W2171123911 created "2016-06-24" @default.
• W2171123911 creator A5051492530 @default.
• W2171123911 creator A5067830382 @default.
• W2171123911 creator A5069373500 @default.
• W2171123911 date "2014-04-01" @default.
• W2171123911 modified "2023-10-16" @default.
• W2171123911 title "CC Coupling of N-Heterocycles at the<i>fac</i>-Re(CO)₃Fragment: Synthesis of Pyridylimidazole and Bipyridine Ligands" @default.
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• W2171123911 doi "https://doi.org/10.1002/chem.201400155" @default.
• W2171123911 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24692049" @default.
• W2171123911 hasPublicationYear "2014" @default.
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