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- W2171990410 abstract "Abstract The reaction of Li/Cl P ‐CPh 3 phosphinidenoid tungsten(0) complex 2 with dimethylcyanamide afforded tricyclic phosphirane complex 4 , an unprecedented rearrangement of which led to the novel N,P,C cage complex 6 . On the basis of DFT calculations, formation and intramolecular [3+2] cycloaddition of the transient nitrilium phosphane ylide complex 3 to a phenyl ring of the triphenylmethyl substituent to give 4 is proposed. Furthermore, theoretical evidence for terminal N ‐amidinophosphinidene complex 7 , formed by [2+1] cycloelimination from 4 , is provided, and the role of the electronic structure and non‐covalent interactions of intermediate 7 discussed." @default.
- W2171990410 created "2016-06-24" @default.
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- W2171990410 date "2014-04-15" @default.
- W2171990410 modified "2023-10-18" @default.
- W2171990410 title "A Novel N,P,C Cage Complex Formed by Rearrangement of a Tricyclic Phosphirane Complex: On the Importance of Non-covalent Interactions" @default.
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- W2171990410 doi "https://doi.org/10.1002/chem.201305061" @default.
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