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• W2174996849 abstract "We report several ruthenium catalysts incorporating mixed donor phosphine-amine ligands for the upgrade of ethanol to the advanced biofuel n-butanol, which show high selectivity (≥90%) at good (up to 31%) conversion. In situ formation of catalysts from mixtures of [RuCl2(η6-p-cymene)]2 and 2-(diphenylphosphino)ethylamine (1) shows enhanced activity at initial water concentrations higher than those of our previously reported diphosphine systems. Preliminary mechanistic studies (electrospray ionization mass spectrometry and nuclear magnetic resonance spectroscopy) suggest the possibility of ligand-assisted proton transfer in some derivatives." @default.
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• W2174996849 date "2015-09-02" @default.
• W2174996849 modified "2023-10-07" @default.
• W2174996849 title "Catalytic Conversion of Ethanol to <i>n</i>-Butanol Using Ruthenium P–N Ligand Complexes" @default.
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• W2174996849 doi "https://doi.org/10.1021/acscatal.5b01327" @default.
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