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- W2181330407 abstract "Abstract This article presents a comprehensive study of the photophysics of 2‐(2‐pyrenylethynyl) adenosine and 2‐(4‐pyrenylethynyl) adenosine, which are structural isomers of the well‐established fluorescent RNA label 2‐(1‐pyrenylethynyl) adenosine. We performed steady‐state and ultrafast transient absorption spectroscopy studies along with time‐resolved fluorescence emission experiments in different solvents to work out the interplay of locally excited and charge‐transfer states. We found the ultrafast photodynamics to be crucial for the fluorescence decay behavior, which extends up to tens of nanoseconds and is partially multi‐exponential. These features in the ultrafast dynamics are indicative of the rotational energy barriers in the first excited state." @default.
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- W2181330407 date "2016-01-13" @default.
- W2181330407 modified "2023-09-26" @default.
- W2181330407 title "The Three Possible 2-(Pyrenylethynyl) Adenosines: Rotameric Energy Barriers Govern the Photodynamics of These Structural Isomers" @default.
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- W2181330407 doi "https://doi.org/10.1002/cphc.201500958" @default.
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