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- W2182578448 abstract "The expected weapons-usable plutonium feed streams to be incorporated in a titanate ceramic immobilization form contain a variety of impurities. One of the goals of the Product Control Model currently under development is to provide a means of projecting the phase assemblage of the ceramic from a knowledge of the feed stream composition. The approach being taken is to develop an understanding of the phase equilibria of the baseline ceramic (without impurities) and then to quantify the effects of impurity additions. In the work reported here, several relevant ternary phase diagrams have been developed by electron microprobe characterization of samples having a wide range of compositions related to the baseline composition. In this work, cerium and thorium were used as surrogates for plutonium. Also characterized are a large number of samples having excess amounts of expected impurities. Results of the phase diagram development show that the approach of using phase equilibria is a promising basis for projecting mineralogy of the plutonium immobilization ceramic. The impurity studies provide limits of solubility of the impurities in the baseline phases and indicate the identity and composition of accessory phases that are formed when impurities are present in excess. Results of the impurity studies show that the ceramic is able to incorporate significant amounts of most of the expected impurities. Those with low solubilities can be controlled by waste stream selection and blending." @default.
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- W2182578448 date "2000-01-01" @default.
- W2182578448 modified "2023-09-27" @default.
- W2182578448 title "PHASE EQUILIBRIA AND EFFECTS OF IMPURITIES ON THE CERAMIC PLUTONIUM IMMOBILIZATION FORM i" @default.
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